Anisotropic high-harmonic generation in bulk crystals

Semiclassical analysis of high harmonic generation in bulk crystals

High harmonic generation (HHG) in solids is investigated. We find that interband emission is dominant for the midinfrared laser driver frequencies, whereas intraband emission dominates the far-infrared range. Interband HHG is similar to atomic HHG and therewith opens the possibility to apply atomic attosecond technology to the condensed matter phase. Interband emission is investigated with a qu...

Surface plasmon-driven second-harmonic generation asymmetry in anisotropic plasmonic crystals

Second harmonic generation from the ‘centrosymmetric’ crystals

Second harmonic generation (SHG) is a well known non-linear optical phenomena which can be observed only in non-centrosymmetric crystals due to non-zero hyperpolarizability. In the current work we observed SHG from a Zn(II) complex which was originally thought to have crystallized in the centrosymmetric space group C2/c. This has been attributed to the unequal antiparallel packing of the metal ...

Tailoring Čerenkov second-harmonic generation in bulk nonlinear photonic crystal.

We investigate theoretically the Čerenkov-type second-harmonic generation in two-dimensional bulk nonlinear photonic crystal with longitudinal modulation of the χ((2)) nonlinearity. We show that in this scheme the Čerenkov radiation can be achieved simultaneously at multiple directions with comparable intensities. The angles of emission are controllable by the spatial modulation of the nonlinea...

Anisotropic magnetization-induced second harmonic generation in FeÕAu superlattices